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This book is a systematic compilation of the most recent body of knowledge in the rapidly developing research area of greenhouse gas interaction with clay systems. Unexpected results of the most recent studies - such as unusually high sorption capacity and sorption hysteresis of swelling clays -stimulated theoretical activity in this fascinating field. Classical molecular dynamics (MD) explains swelling caused by intercalation of water molecules and to a certain degree of CO2 molecules in clay interlayer. However, unusual frequency shifts in the transient infrared fingerprints of the...