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The focus of this thesis is the interplay of synchrony and adaptivity in complex networks. Synchronization is a ubiquitous phenomenon observed in different contexts in physics, chemistry, biology, neuroscience, medicine, socioeconomic systems, and engineering. Most prominently, synchronization takes place in the brain, where it is associated with cognitive capacities like learning and memory, but is also a characteristic of neurological diseases like Parkinson and epilepsy. Adaptivity is common in many networks in nature and technology, where the connectivity changes in time, i.e., the...