This monograph provides a state-of-the-art treatment of learning and robust control in quantum technology. It presents a systematic investigation of control design and algorithm realisation for several classes of quantum systems using control-theoretic tools and machine-learning methods. The approaches rely heavily on examples and the authors cover:sliding mode control of quantum systems;control and classification of inhomogeneous quantum ensembles using sampling-based learning control;robust and optimal control design using machine-learning methods;robust stability of quantum systems;...