This monograph reviews the establishment of new theories of the ozone hole and global climate change, two major scientific problems of global concern. It provides a comprehensive overview of the author's work including significant discoveries and pioneering contributions, such as the discovery of extremely effective dissociative electron transfer reactions of chlorofluorocarbons (CFCs) adsorbed on ice surfaces and its implications for atmospheric ozone depletion; the proposal of the cosmic-ray-driven electron-induced-reaction (CRE) theory for the ozone hole; the predictions of the existence...