Preface.- Introduction: Chemistry of the Troposphere — Some Problems and Their Temporal Frameworks.- Factors Governing the pH, Availability of H+, and Oxidation Capacity of Rain.- The Chemical Composition of Precipitation: A Southern Hemisphere Perspective.- Some Influences of the Atmospheric Water Cycle on the Removal of Atmospheric Trace Constituents.- Aqueous Chemistry in the Atmosphere.- The History of Atmospheric Composition As Recorded in Ice Sheets.- Lake and Wetland Sediments As Records of Past Atmospheric Composition.- The History of the Atmosphere As Recorded by Carbon Isotopes.- Changes in Atmospheric Composition.- The Production and Fate of Reduced Volatile Species from Oxic Environments.- The Production and Fate of Reduced C, N, and S Gases from Oxygen-deficient Environments.- The Production and Fate of Volatile Molecular Species in the Environment: Metals and Metalloids.- Biogenic Contributions to Atmospheric Chemistry.- Physics and Chemistry of Atmospheric Ions.- Homogeneous Gas Phase Oxidation Processes in the Troposphere.- The Global Distribution of Hydroxyl.- Non-methane Organics in the Remote Troposphere.- Tropospheric Gases, Aerosols and Photochemical Reactions.- List of Participants.- Author Index.